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High coke-resistance Pt/Mg1-xNixO catalyst for dry reforming of methane


Citation

Al-Doghachi, Faris A. J. and Islam, Aminul and Zainal, Zulkarnain and Saiman, Mohd Izham and Embong, Zaidi and Yap, Taufiq Yun Hin (2016) High coke-resistance Pt/Mg1-xNixO catalyst for dry reforming of methane. PLOS ONE, 11 (1). art. no. e0145862. pp. 1-22. ISSN 1932-6203

Abstract / Synopsis

A highly active and stable nano structured Pt/Mg1-xNixO catalysts was developed by a simple co-precipitation method. The obtained Pt/Mg1-xNixO catalyst exhibited cubic structure nanocatalyst with a size of 50–80 nm and realized CH4 and CO2 conversions as high as 98% at 900°C with excellent stability in the dry reforming of methane. The characterization of catalyst was performed using various kinds of analytical techniques including XRD, BET, XRF, TPR-H2, TGA, TEM, FESEM, FT-IR, and XPS analyses. Characterization of spent catalyst further confirms that Pt/Mg1-xNixO catalyst has high coke-resistance for dry reforming. Thus, the catalyst demonstrated in this study, offers a promising catalyst for resolving the dilemma between dispersion and reducibility of supported metal, as well as activity and stability during high temperature reactions.


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Additional Metadata

Item Type: Article
Divisions: Faculty of Science
DOI Number: https://doi.org/10.1371/journal.pone.0145862
Publisher: Public Library of Science
Keywords: Pt/Mg1-xNixO; High coke-resistance
Depositing User: Nabilah Mustapa
Date Deposited: 08 Jun 2016 12:22
Last Modified: 08 Jun 2016 12:22
Altmetrics: http://www.altmetric.com/details.php?domain=psasir.upm.edu.my&doi=10.1371/journal.pone.0145862
URI: http://psasir.upm.edu.my/id/eprint/17107
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